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Uranium from German Nuclear Power Projects of the 1940s - A Nuclear Forensic Investigation

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Authors

Mayer, Klaus
Wallenius, M.
Lutzenkirchen, Klaus
Horta, Joan
Nicholl, Adrian
Rasmussen, Gert
van Belle, Pieter
Varga, Z.
Buda, Razvan
Erdmann, Nicole

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Wiley-VCH Verlag GMBH

Abstract

Abstract: Here we present a nuclear forensic study of uranium from German nuclear projects which used different geometries of metallic uranium fuel.[3b,d, 4] Through measurement of the 230Th/234U ratio, we could determine that the material had been produced in the period from 1940 to 1943. To determine the geographical origin of the uranium, the rare-earth-element content and the 87Sr/86Sr ratio were measured. The results provide evidence that the uranium was mined in the Czech Republic. Trace amounts of 236U and 239Pu were detected at the level of their natural abundance, which indicates that the uranium fuel was not exposed to any major neutron fluence

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Source

Angewandte Chemie International Edition

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Restricted until

2037-12-31
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