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Resonant Raman scattering from silicon nanoparticles enhanced by magnetic response

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Dmitriev, Pavel A.
Baranov, Denis G.
Milichko, Valentin A.
Makarov, Sergey V.
Mukhin, Ivan S.
Samusev, Anton K.
Krasnok, Alexander E.
Belov, Pavel A.
Kivshar, Yuri

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Royal Society of Chemistry

Abstract

Enhancement of optical response with high-index dielectric nanoparticles is attributed to the excitation of their Mie-type magnetic and electric resonances. Here we study Raman scattering from crystalline silicon nanoparticles and reveal that magnetic dipole modes have a much stronger effect on the scattering than electric modes of the same order. We demonstrate experimentally a 140-fold enhancement of the Raman signal from individual silicon spherical nanoparticles at the magnetic dipole resonance. Our results confirm the importance of the optically-induced magnetic response of subwavelength dielectric nanoparticles for enhancing light-matter interactions.

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Nanoscale

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