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Aqueous electrochemistry of the magnesium surface: Thermodynamic and kinetic profiles

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dc.contributor.authorYuwono, Jodie A.
dc.contributor.authorBirbilis, Nick
dc.contributor.authorTaylor, Christopher D.
dc.contributor.authorWilliams, Kristen S.
dc.contributor.authorSamin, Adib J.
dc.contributor.authorMedhekar, Nikhil
dc.date.accessioned2020-03-16T00:16:34Z
dc.date.issued2019
dc.date.updated2019-11-25T07:42:02Z
dc.description.abstractIn this study, first-principles density functional theory (DFT) calculations are performed to investigate the contribution of each individual reaction at the magnesium/water interface. Thermodynamic and kinetic models derived from the DFT-calculated parameters are used to describe interdependent reactions at the interface and the resultant magnesium electrochemical activity at different pH and potentials. These models are able to rationalise experimental findings, such as those obtained from polarisation and immersion tests, and provide new insights for defining a complete and viable mechanism of aqueous magnesium electrochemistry.en_AU
dc.description.sponsorshipJ.A.Y received funding from the Monash International Postgraduate Scholarship (MIPRS), Monash Graduate Scholarship (MGS), Monash Study Away/ Travel Grant and Graduate Research International Travel Award (GRITA). N.B and N.V.M received funding from Australian Research Council DP Scheme (DP160103661). N.B. received support by Woodside Energy.en_AU
dc.format.mimetypeapplication/pdfen_AU
dc.identifier.issn0010-938Xen_AU
dc.identifier.urihttp://hdl.handle.net/1885/202218
dc.language.isoen_AUen_AU
dc.provenancehttp://sherpa.ac.uk/romeo/issn/0010-938X/..."Author's post-print on open access repository after an embargo period of 24 months. Author's post-print must be released with a Creative Commons Attribution Non-Commercial No Derivatives License" from SHERPA/RoMEO site (as at 18/03/2020).
dc.publisherElsevieren_AU
dc.relationhttp://purl.org/au-research/grants/arc/DP160103661en_AU
dc.rights© 2018 Elsevier Ltden_AU
dc.rights.licenseCreative Commons Attribution Non-Commercial No Derivatives License
dc.rights.urihttps://creativecommons.org/licenses/by-nc-nd/4.0/
dc.sourceCorrosion Scienceen_AU
dc.titleAqueous electrochemistry of the magnesium surface: Thermodynamic and kinetic profilesen_AU
dc.typeJournal articleen_AU
dcterms.accessRightsOpen Access
local.bibliographicCitation.lastpage68en_AU
local.bibliographicCitation.startpage53en_AU
local.contributor.affiliationYuwono, Jodie A., Monash Universityen_AU
local.contributor.affiliationBirbilis, Nick, College of Engineering and Computer Science, ANUen_AU
local.contributor.affiliationTaylor, Christopher D., The Ohio State Universityen_AU
local.contributor.affiliationWilliams, Kristen S., Boeing Research and Technologyen_AU
local.contributor.affiliationSamin, Adib J., Los Alamos National Laboratoryen_AU
local.contributor.affiliationMedhekar, Nikhil, Monash Universityen_AU
local.contributor.authoruidBirbilis, Nick, u1066695en_AU
local.description.notesImported from ARIESen_AU
local.identifier.absfor091207 - Metals and Alloy Materialsen_AU
local.identifier.absfor091299 - Materials Engineering not elsewhere classifieden_AU
local.identifier.absseo861206 - Structural Metal Productsen_AU
local.identifier.absseo861199 - Basic Metal Products not elsewhere classifieden_AU
local.identifier.ariespublicationu3102795xPUB439en_AU
local.identifier.citationvolume147en_AU
local.identifier.doi10.1016/j.corsci.2018.10.014en_AU
local.identifier.scopusID2-s2.0-85056787644
local.publisher.urlhttps://www.elsevier.com/en-auen_AU
local.type.statusAccepted Versionen_AU

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