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Discovery and Synthesis of Boletopsins 13 and 14, Brominated Fungal Metabolites of Terrestrial Origin

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dc.contributor.authorBeekman, Andrew
dc.contributor.authorWossa, Stewart
dc.contributor.authorKevo, Oromo
dc.contributor.authorMa, Paul
dc.contributor.authorBarrow, Russell
dc.date.accessioned2016-06-14T23:20:09Z
dc.date.issued2015
dc.date.updated2016-06-14T08:46:16Z
dc.description.abstractHere we report the discovery and synthesis of complex polybrominated p-terphenyl ethers isolated from a mushroom (Boletopsis sp.) used as a traditional medicine by the Kiovi people in the highlands of Papua New Guinea. Boletopsins 13 and 14 represent the first report of polybrominated fungal metabolites to be produced by a terrestrial fungus. The synthetic method employs 2,4,4,6-tetrabromo-2,5-cyclohexadienone to achieve selective polybromination of the extended aromatic system in a selective and sequential manner. (Chemical Equation Presented).
dc.identifier.issn0163-3864
dc.identifier.urihttp://hdl.handle.net/1885/103234
dc.publisherAmerican Chemical Society
dc.sourceJournal of Natural Products
dc.titleDiscovery and Synthesis of Boletopsins 13 and 14, Brominated Fungal Metabolites of Terrestrial Origin
dc.typeJournal article
local.bibliographicCitation.issue8
local.bibliographicCitation.lastpage2135
local.bibliographicCitation.startpage2133
local.contributor.affiliationBeekman, Andrew, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationWossa, Stewart, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationKevo, Oromo, Kiovi Village, Lufa District
local.contributor.affiliationMa, Paul, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationBarrow, Russell, College of Physical and Mathematical Sciences, ANU
local.contributor.authoruidBeekman, Andrew, u4311066
local.contributor.authoruidWossa, Stewart, u4472724
local.contributor.authoruidMa, Paul, u4532622
local.contributor.authoruidBarrow, Russell, u9902002
local.description.embargo2037-12-31
local.description.notesImported from ARIES
local.identifier.absfor030502 - Natural Products Chemistry
local.identifier.absfor030503 - Organic Chemical Synthesis
local.identifier.absfor060500 - MICROBIOLOGY
local.identifier.absseo970103 - Expanding Knowledge in the Chemical Sciences
local.identifier.ariespublicationU3488905xPUB5746
local.identifier.citationvolume78
local.identifier.doi10.1021/acs.jnatprod.5b00202
local.identifier.scopusID2-s2.0-84940513580
local.type.statusPublished Version

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