Observation of the dynamic Jahn-Teller effect in the excited states of nitrogen-vacancy centers in diamond
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Fu, Kai-Mei C
Santori, Charles
Barclay, Paul E.
Rogers, Lachlan
Manson, Neil
Beausoleil, R.
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American Physical Society
Abstract
The optical transition linewidth and emission polarization of single nitrogen-vacancy (NV) centers are measured from 5 K to room temperature. Interexcited state population relaxation is shown to broaden the zero-phonon line and both the relaxation and linewidth are found to follow a T5 dependence for T<100K. This dependence indicates that the dynamic Jahn-Teller effect is the dominant dephasing mechanism for the NV optical transitions at low temperatures.
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Physical Review Letters
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2037-12-31
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