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Synthesis of an expanded pincer ligand and its bimetallic coinage metal complexes

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dc.contributor.authorDelaney, Andie
dc.contributor.authorYu, Li-Juan
dc.contributor.authorCoote, Michelle
dc.contributor.authorColebatch, Annie
dc.date.accessioned2023-10-09T03:44:58Z
dc.date.available2023-10-09T03:44:58Z
dc.date.issued2021
dc.date.updated2022-11-13T07:16:34Z
dc.description.abstractAn expanded pincer ligand tBu-PONNOP (2,7-bis(di-tert-butylphosphinito)-1,8-naphthyridine) has been synthesised and its coordination to coinage metals has been studied. Bimetallic complexes were produced with metal halide salts of the type [M2X2(tBu-PONNOP)] (X = Cl, M = Au, Ag, Cu; X = I, M = Cu) with a varying degree of interaction with the naphthyridyl backbone in the order Au < Ag < Cu. The salts [Ag-2(tBu-PONNOP)(2)][BAr4F](2) (Ar-F = 3,5-C6H3(CF3)(2)) and [Ag-2(NCMe)(2)(tBu-PONNOP)]X-2 (X = BAr4F, PF6) were prepared, which may serve as a source of tBu-PONNOP via transmetallation.en_AU
dc.description.sponsorshipFinancial support from the Australian Research Council (A.L.C. DECRA Fellowship DE200100450, M.L.C. Laureate Fellowship FL170100041) and Westpac (A.R.D. Future Leaders Scholarship).en_AU
dc.format.mimetypeapplication/pdfen_AU
dc.identifier.issn1477-9226en_AU
dc.identifier.urihttp://hdl.handle.net/1885/301812
dc.language.isoen_AUen_AU
dc.provenancehttps://v2.sherpa.ac.uk/id/publication/18010..."Author Accepted Manuscript can be made open access on institutional repository after 12 month embargo" from SHERPA/RoMEO site (as at 9.10.2023).en_AU
dc.publisherRoyal Society of Chemistryen_AU
dc.relationhttp://purl.org/au-research/grants/arc/DE200100450en_AU
dc.relationhttp://purl.org/au-research/grants/arc/FL170100041en_AU
dc.rights© 2021 The Royal Society of Chemistryen_AU
dc.sourceDalton Transactionsen_AU
dc.titleSynthesis of an expanded pincer ligand and its bimetallic coinage metal complexesen_AU
dc.typeJournal articleen_AU
dcterms.accessRightsOpen Accessen_AU
dcterms.dateAccepted2021-08-05
local.bibliographicCitation.issue34en_AU
local.bibliographicCitation.lastpage11917en_AU
local.bibliographicCitation.startpage11909en_AU
local.contributor.affiliationDelaney, Andie, College of Science, ANUen_AU
local.contributor.affiliationYu, Lijuan, College of Science, ANUen_AU
local.contributor.affiliationCoote, Michelle, College of Science, ANUen_AU
local.contributor.affiliationColebatch, Annie, College of Science, ANUen_AU
local.contributor.authoruidDelaney, Andie, u6046179en_AU
local.contributor.authoruidYu, Lijuan, u1055437en_AU
local.contributor.authoruidCoote, Michelle, u4031074en_AU
local.contributor.authoruidColebatch, Annie, u4213195en_AU
local.description.notesImported from ARIESen_AU
local.identifier.absfor340211 - Transition metal chemistryen_AU
local.identifier.absfor340209 - Organometallic chemistryen_AU
local.identifier.ariespublicationa383154xPUB21152en_AU
local.identifier.citationvolume50en_AU
local.identifier.doi10.1039/d1dt01741aen_AU
local.identifier.thomsonIDWOS:000683438200001
local.publisher.urlhttps://pubs.rsc.org/en_AU
local.type.statusAccepted Versionen_AU

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