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Experimental verification of line- and band-shape asymmetry in the Schumann–Runge system of O[sub 2]

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dc.contributor.authorKono, Men_AU
dc.contributor.authorLewis, B. Ren_AU
dc.contributor.authorGibson, S. Ten_AU
dc.contributor.authorBaldwin, Kennethen_AU
dc.date.accessioned2015-10-08T22:49:20Z
dc.date.available2015-10-08T22:49:20Z
dc.date.created22/06/2003en_AU
dc.date.issued2003en_AU
dc.date.updated2015-12-12T08:17:32Z
dc.description.abstractHigh-resolution, laser-based photoabsorption cross-section measurements in the weakly absorbing windows between the (11,0) and (16,0) Schumann–Runge bands of O₂ have been performed at liquid-nitrogen temperature and the results compared with corresponding coupled-channel Schrödinger-equation (CSE) and line-by-line model calculations. While the symmetric-line- shape-based line-by-line model cross sections differ significantly from experiment, the excellent agreement found between the CSE and experimental window cross sections serves to confirm clearly for the first time the CSE-model predictions of band shape asymmetry and quantum-mechanical interference effects, especially in the (11,0)–(14,0) band region.
dc.format.extent1 vol.en_AU
dc.format.mimetypeapplication/pdfen_AU
dc.identifier.issn0021-9606en_AU
dc.identifier.urihttp://hdl.handle.net/1885/15826
dc.language.isoen_AUen_AU
dc.publisherAmerican Institute of Physics (AIP)en_AU
dc.sourceThe Journal of Chemical Physicsen_AU
dc.subjectKeywords: Laser applications; Photodissociation; Photons; Ultraviolet radiation; Quantum-mechanical interference effects; Quantum theoryen_AU
dc.titleExperimental verification of line- and band-shape asymmetry in the Schumann–Runge system of O[sub 2]en_AU
dc.typeJournal articleen_AU
local.bibliographicCitation.issue24en_AU
local.bibliographicCitation.lastpage10928en_AU
local.bibliographicCitation.startpage10924en_AU
local.contributor.affiliationKono, Mitsuhiko, College of Physical and Mathematical Sciences, CPMS Research School of Physics and Engineering, Atomic and Molecular Physics Laboratories, The Australian National Universityen_AU
local.contributor.affiliationLewis, Brenton, College of Physical and Mathematical Sciences, CPMS Research School of Physics and Engineering, Atomic and Molecular Physics Laboratories, The Australian National Universityen_AU
local.contributor.affiliationBaldwin, Kenneth, College of Physical and Mathematical Sciences, CPMS Research School of Physics and Engineering, Laser Physics Centre, The Australian National Universityen_AU
local.contributor.affiliationGibson, Stephen, College of Physical and Mathematical Sciences, CPMS Research School of Physics and Engineering, Atomic and Molecular Physics Laboratories, The Australian National Universityen_AU
local.contributor.authoruidu4030223en_AU
local.description.notesImported from ARIESen_AU
local.description.refereedYes
local.identifier.absfor020201 - Atomic and Molecular Physicsen_AU
local.identifier.ariespublicationMigratedxPub15881en_AU
local.identifier.citationvolume118en_AU
local.identifier.doi10.1063/1.1574512en_AU
local.identifier.scopusID2-s2.0-0038793540
local.publisher.urlhttps://www.aip.org/en_AU
local.type.statusPublished Versionen_AU

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