Carrier Lifetime and Mobility Enhancement in Nearly Defect-Free Core-Shell Nanowires Measured Using Time-Resolved Terahertz Spectroscopy

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Parkinson, Patrick Wallace
Joyce, Hannah J
Gao, Qiang
Zhang, Xin
Jagadish, Chennupati
Herz, Laura
Johnston, Michael B
Tan, Hark Hoe

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American Chemical Society

Abstract

We have used transient terahertz photoconductivity measurements to assess the efficacy of two-temperature growth and core-shell encapsulation techniques on the electronic properties of GaAs nanowires. We demonstrate that two-temperature growth of the GaAs core leads to an almost doubling in charge-carrier mobility and a tripling of carrier lifetime. In addition, overcoating the GaAs core with a larger-bandgap material is shown to reduce the density of surface traps by 82%, thereby enhancing the charge conductivity.

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Nano Letters

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Restricted until

2037-12-31