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Two-photon absorption properties of multipolar triarylamino/tosylamido 1,1,4,4-tetracyanobutadienes

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dc.contributor.authorRipoche, Nicholas
dc.contributor.authorBetou, Marie
dc.contributor.authorPhilippe, Clotilde
dc.contributor.authorTrolez, Yann
dc.contributor.authorMongin, Olivier
dc.contributor.authorDudek, Marta
dc.contributor.authorPokladek, Ziemowit
dc.contributor.authorMatczyszyn, Katarzyna
dc.contributor.authorSamoc, Marek
dc.contributor.authorSahnoune, Hiba
dc.contributor.authorHalet, Jean-Francois
dc.contributor.authorRoisnel, Thierry
dc.contributor.authorToupet, Loic
dc.contributor.authorCordier, Marie-Odile
dc.contributor.authorMoxey, Graeme
dc.contributor.authorHumphrey, Mark
dc.contributor.authorPaul, Frederic
dc.date.accessioned2024-03-18T22:21:49Z
dc.date.issued2021
dc.date.updated2022-11-13T07:17:07Z
dc.description.abstractThe synthesis and characterization of four new tetracyanobutadiene (TCBD) derivatives (1,3cand4b-c) incorporating tosylamido and 4-triphenylamino moieties are reported. Along with those of five closely related or differently branched TCBDs derivatives (2,3a-b,4cand5), their linear and (third-order) nonlinear optical properties were investigated by electronic absorption spectroscopy and Z-scan measurements. Among these compounds, the tri-branched compounds3cand5are the most active two-photon absorbers, with effective cross-sections of 275 and 350 GM at 900 nm, respectively. These properties are briefly discussed with the help of DFT calculations, focussing on structural and electronic factors, and contextualized with results obtained previously for related compounds.en_AU
dc.description.sponsorshipThis research was supported by grants from Campus France (PHC Polonium Program 2017 No. 37629XG), the National Science Centre of Poland (NCN Opus UMO-2019/35/B/ST4/ 03280 and Harmonia UMO-2016/22/M/ST4/00275, Wroclaw University of Science and Technology), the Erasmus Plus program (M. D. and Z. P.), the CNRS (PICS programs No. 5676 & 7106 and LIA Redochrom), the ‘‘Region Bretagne’’ (N. R., M. B. and C. P), theAgenceNationalepour laRecherche (JCJC Fluotet 17-CE070038-01).Calculations were carried out at the Wroclaw Centre for Networking and Supercomputing and at the local computing center from the ISCR (France). H. S. acknowledges the Algerian PRFU project (2020-2024: Grant No. B00L01UN3501202-00003).en_AU
dc.format.mimetypeapplication/pdfen_AU
dc.identifier.issn1463-9076en_AU
dc.identifier.urihttp://hdl.handle.net/1885/316088
dc.language.isoen_AUen_AU
dc.publisherRoyal Society of Chemistryen_AU
dc.relationhttp://purl.org/au-research/grants/arc/DP170100408en_AU
dc.rights© 2021 The authorsen_AU
dc.sourcePhysical Chemistry Chemical Physicsen_AU
dc.titleTwo-photon absorption properties of multipolar triarylamino/tosylamido 1,1,4,4-tetracyanobutadienesen_AU
dc.typeJournal articleen_AU
local.bibliographicCitation.issue39en_AU
local.bibliographicCitation.lastpage22297en_AU
local.bibliographicCitation.startpage22283en_AU
local.contributor.affiliationRipoche, Nicholas, College of Science, ANUen_AU
local.contributor.affiliationBetou, Marie, Nationale Supérieure de Chimie de Rennes CNRSen_AU
local.contributor.affiliationPhilippe, Clotilde, Institut des Sciences Chimiques de Rennesen_AU
local.contributor.affiliationTrolez, Yann, Nationale Supérieure de Chimie de Rennes CNRSen_AU
local.contributor.affiliationMongin, Olivier, Universite Rennesen_AU
local.contributor.affiliationDudek, Marta, Wroclaw University of Science and Technologyen_AU
local.contributor.affiliationPokladek, Ziemowit, Wroclaw University of Science and Technologyen_AU
local.contributor.affiliationMatczyszyn, Katarzyna, Wroclaw UniVersity of Technologyen_AU
local.contributor.affiliationSamoc, Marek, College of Science, ANUen_AU
local.contributor.affiliationSahnoune, Hiba, Universite´ M’Hamed Bouguara de Boumerdesen_AU
local.contributor.affiliationHalet, Jean-Francois, Universite de Rennesen_AU
local.contributor.affiliationRoisnel, Thierry, Institut des Sciences Chimiques de Rennesen_AU
local.contributor.affiliationToupet, Loic, Universite de Rennesen_AU
local.contributor.affiliationCordier, Marie-Odile, Universite de Rennesen_AU
local.contributor.affiliationMoxey, Graeme, College of Science, ANUen_AU
local.contributor.affiliationHumphrey, Mark, College of Science, ANUen_AU
local.contributor.affiliationPaul, Frederic, Universite de Rennesen_AU
local.contributor.authoruidRipoche, Nicholas, u5306966en_AU
local.contributor.authoruidSamoc, Marek, u9115357en_AU
local.contributor.authoruidMoxey, Graeme, u5200340en_AU
local.contributor.authoruidHumphrey, Mark, u9400918en_AU
local.description.embargo2099-12-31
local.description.notesImported from ARIESen_AU
local.identifier.absfor340304 - Optical properties of materialsen_AU
local.identifier.ariespublicationa383154xPUB22655en_AU
local.identifier.citationvolume23en_AU
local.identifier.doi10.1039/d1cp03346hen_AU
local.identifier.scopusID2-s2.0-85117233599
local.identifier.thomsonIDWOS:000700908500001
local.publisher.urlhttps://pubs.rsc.org/en_AU
local.type.statusPublished Versionen_AU

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