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Total Synthesis of Suillusin

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Date

2018

Authors

Zhang, Meng Yao
Malins, Lara
Ward, James
Barrow, Russell A

Journal Title

Journal ISSN

Volume Title

Publisher

American Chemical Society

Abstract

The first total synthesis of the fungal natural product suillusin is reported. The key features of the synthesis include a Michael-benzoin multicatalytic cascade that assembles the entire carbon framework in a single step, and a Rubottom-Swern oxidation sequence that yields the requisite diketone oxidation state of the core framework. This 10-step synthesis of suillusin will allow further evaluation of the biogenesis and the biological activity of the fungal metabolite.

Description

Keywords

Citation

URI

http://hdl.handle.net/1885/256641

Collections

ANU Research Publications

Source

Organic Letters

Type

Journal article

Book Title

Entity type

Access Statement

License Rights

DOI

10.1021/acs.orglett.8b03234

Restricted until

2099-12-31

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01_Zhang_Total_Synthesis_of_Suillusin_2018.pdf (1.2 MB)

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