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Organometallic Complexes for Nonlinear Optics, 47 - Synthesis and Cubic Optical Nonlinearity of a Stilbenylethynylruthenium Dendrimer

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dc.contributor.authorJeffery, Christopher
dc.contributor.authorCifuentes, Marie
dc.contributor.authorDalton, Gulliver
dc.contributor.authorCorkery, Timothy
dc.contributor.authorRandles , Michael
dc.contributor.authorWillis, Anthony
dc.contributor.authorSamoc, Marek
dc.contributor.authorHumphrey, Mark
dc.date.accessioned2015-12-10T22:54:58Z
dc.date.issued2010
dc.date.updated2016-02-24T10:43:56Z
dc.description.abstract(Figure Presented) The synthesis of the 1st generation dendrimer l,3,5-{trans-[Ru(C=C-3,5-(trans-[Ru(C= CPh)(dppe)2(C=CC 6H4-4-(E)-CH=CH)] )2C6H 3)(dppe)2(C=CC6H4-4-(E)-CH=CH)] }3C6H3 proceeds by a novel route that features Emmons-Horner-Wadsworth coupling of 1,3,5-C6H3(CH 2PO(OEt)2)3 with trans-[Ru(C≡CC 6H4-4CHO)Cl(dppe)2] and 1-I-C6H 3-3,5-(CH2PO(OEt)2)2 with trans-[Ru(C≡CPh)(C≡CC6H4-4-CHO)(dppe) 2] as key steps. The stilbenylethynylruthenium dendrimer is much more soluble than its ethynylated analog l,3,5-{trans-[Ru(C≡C-3,5-(trans- [Ru(C≡CPh) (dppe)2(C≡CC6H4-4- C≡C)] )2C6H3)(dppe)2(C≡ CC6H44-C≡C)] }3C6H3 and, in contrast to the ethynylated analog, is a two-photon absorber at telecommunications wavelengths.
dc.identifier.issn1022-1336
dc.identifier.urihttp://hdl.handle.net/1885/59885
dc.publisherWiley-VCH Verlag GMBH
dc.sourceMacromolecular Rapid Communications
dc.subjectKeywords: Cubic optical nonlinearity; Inorganic materials; NLO; Novel route; Organometallic complex; TEM; Two photon; Dendrimers; Lanthanum compounds; Nonlinear optics; Organometallics; Synthesis (chemical); Crystal structure Crystal structure; Dendrimers; Inorganic materials; NLO; TEM
dc.titleOrganometallic Complexes for Nonlinear Optics, 47 - Synthesis and Cubic Optical Nonlinearity of a Stilbenylethynylruthenium Dendrimer
dc.typeJournal article
local.bibliographicCitation.issue9-10
local.bibliographicCitation.lastpage849
local.bibliographicCitation.startpage846
local.contributor.affiliationJeffery, Christopher, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationCifuentes, Marie, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationDalton, Gulliver, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationCorkery, Timothy, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationRandles , Michael , College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationWillis, Anthony, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationSamoc, Marek, Wroclaw University of Technology
local.contributor.affiliationHumphrey, Mark, College of Physical and Mathematical Sciences, ANU
local.contributor.authoruidJeffery, Christopher, u3375413
local.contributor.authoruidCifuentes, Marie, u9410034
local.contributor.authoruidDalton, Gulliver, u3170420
local.contributor.authoruidCorkery, Timothy, u4261121
local.contributor.authoruidRandles , Michael , u3956935
local.contributor.authoruidWillis, Anthony, u8512028
local.contributor.authoruidHumphrey, Mark, u9400918
local.description.embargo2037-12-31
local.description.notesImported from ARIES
local.identifier.absfor039904 - Organometallic Chemistry
local.identifier.absseo970103 - Expanding Knowledge in the Chemical Sciences
local.identifier.ariespublicationu4217927xPUB512
local.identifier.citationvolume31
local.identifier.doi10.1002/marc.200900859
local.identifier.scopusID2-s2.0-77952593997
local.identifier.thomsonID000278436300009
local.type.statusPublished Version

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