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Total Syntheses of the Resorcylic Acid Lactone Neocosmosin A and Its Enantiomer

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dc.contributor.authorZhang, Yiwen
dc.contributor.authorDlugosch, Michael
dc.contributor.authorJubermann, Martin
dc.contributor.authorBanwell, Martin
dc.contributor.authorWard, James
dc.date.accessioned2015-12-10T23:11:03Z
dc.date.issued2015
dc.date.updated2015-12-10T09:19:33Z
dc.description.abstractA total synthesis of the structure, 1, assigned to the recently reported resorcylic acid lactone (RAL) neocosmosin A has been established. Olefin-cross metathesis, ring-closing metathesis, palladium-catalyzed Meinwald rearrangement, and Mitsunobu esterification reactions were used as key steps. A late-stage and simple modification to the reaction sequence also provided compound ent-1 that, in fact, represents the true structure of the natural product.
dc.identifier.issn0022-3263
dc.identifier.urihttp://hdl.handle.net/1885/63651
dc.publisherAmerican Chemical Society
dc.sourceJournal of Organic Chemistry
dc.titleTotal Syntheses of the Resorcylic Acid Lactone Neocosmosin A and Its Enantiomer
dc.typeJournal article
local.bibliographicCitation.issue9
local.bibliographicCitation.lastpage4833
local.bibliographicCitation.startpage4828
local.contributor.affiliationZhang, Yiwen, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationDlugosch, Michael, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationJubermann, Martin, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationBanwell, Martin, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationWard, James, College of Physical and Mathematical Sciences, ANU
local.contributor.authoruidZhang, Yiwen, u5293232
local.contributor.authoruidDlugosch, Michael, u5663327
local.contributor.authoruidJubermann, Martin, u5436439
local.contributor.authoruidBanwell, Martin, u9500594
local.contributor.authoruidWard, James, u4431856
local.description.embargo2037-12-31
local.description.notesImported from ARIES
local.identifier.absfor030502 - Natural Products Chemistry
local.identifier.absseo970103 - Expanding Knowledge in the Chemical Sciences
local.identifier.ariespublicationU4217927xPUB832
local.identifier.citationvolume80
local.identifier.doi10.1021/acs.joc.5b00590
local.identifier.scopusID2-s2.0-84928910864
local.type.statusPublished Version

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