High performance Bi₀.₅Na₀.₅TiO₃-BiAlO₃-K₀.₅Na₀.₅NbO₃ lead-free pyroelectric ceramics for thermal detectors
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Liu, Zhen; Peng, Ping; Ren, Weijun; Lu, Teng; Liu, Yun; Guo, Shaobo; Dong, Xianlin; Wang, Genshui
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Both high pyroelectric properties and good temperature stability of ferroelectric materials are desirable when used for applications in infrared thermal detectors. In this work, we report lead-free ternary 0.97(0.99Bi0.5Na0.5TiO3-0.01BiAlO3)-0.03K0.5Na0.5NbO3 (BNT-BA-KNN) ceramics, which not only exhibits a large pyroelectric coefficient (p ∼ 3.7 × 10-8 C cm-2K-1) and figures of merit (Fi, Fv, and Fd) but also shows excellent thermal stable properties. At room temperature, Fi, Fv, and Fd are...[Show more]
dc.contributor.author | Liu, Zhen | |
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dc.contributor.author | Peng, Ping | |
dc.contributor.author | Ren, Weijun | |
dc.contributor.author | Lu, Teng | |
dc.contributor.author | Liu, Yun | |
dc.contributor.author | Guo, Shaobo | |
dc.contributor.author | Dong, Xianlin | |
dc.contributor.author | Wang, Genshui | |
dc.date.accessioned | 2019-07-11T04:05:49Z | |
dc.date.available | 2019-07-11T04:05:49Z | |
dc.identifier.issn | 0003-6951 | |
dc.identifier.uri | http://hdl.handle.net/1885/164537 | |
dc.description.abstract | Both high pyroelectric properties and good temperature stability of ferroelectric materials are desirable when used for applications in infrared thermal detectors. In this work, we report lead-free ternary 0.97(0.99Bi0.5Na0.5TiO3-0.01BiAlO3)-0.03K0.5Na0.5NbO3 (BNT-BA-KNN) ceramics, which not only exhibits a large pyroelectric coefficient (p ∼ 3.7 × 10-8 C cm-2K-1) and figures of merit (Fi, Fv, and Fd) but also shows excellent thermal stable properties. At room temperature, Fi, Fv, and Fd are determined as high as 1.32 × 10-10 m/V, 2.89 × 10-2 m2/C, and 1.15 × 10-5Pa-1/2 at 1 kHz and 1.32 × 10-10 m/V, 2.70 × 10-2 m2/C, and 1.09 × 10-5Pa-1/2 at 20 Hz, respectively. During the temperature range of RT to 85 °C, the achieved p, Fi, Fv, and Fd do not vary too much. The high depolarization temperature and the undispersed ferroelectric-ergodic relaxor phase transition with a sharp pyroelectric coefficient peak value of ∼400 × 10-8 C cm-2K-1 are suggested to be responsible for this thermal stability, which ensures reliable actual operation. The results reveal the BNT-BA-KNN ceramics as promising lead-free candidates for infrared thermal detector applications. | |
dc.description.sponsorship | This work was supported by the Chinese Academy of Sciences Research Equipment Development Project (No. YZ201332), the National Natural Science Foundation (NSFC) of China (No. 61475176), the Shanghai International Science and Technology Cooperation Project (Grant No. 13520700700), and the International Partnership Project of Chinese Academy of Science. Zhen Liu also acknowledges the support of the Shanghai Sailing Program (No. 17YF1429700). | |
dc.format.mimetype | application/pdf | |
dc.language.iso | en_AU | |
dc.publisher | American Institute of Physics | |
dc.rights | © 2018 | |
dc.source | Applied Physics Letters | |
dc.title | High performance Bi₀.₅Na₀.₅TiO₃-BiAlO₃-K₀.₅Na₀.₅NbO₃ lead-free pyroelectric ceramics for thermal detectors | |
dc.type | Journal article | |
local.description.notes | Imported from ARIES | |
local.identifier.citationvolume | 112 | |
dc.date.issued | 2018-04-03 | |
local.identifier.absfor | 030606 - Structural Chemistry and Spectroscopy | |
local.identifier.ariespublication | a383154xPUB9699 | |
local.publisher.url | https://www.aip.org/ | |
local.type.status | Published Version | |
local.contributor.affiliation | Liu, Zhen, College of Science, ANU | |
local.contributor.affiliation | Peng, Ping, Chinese Academy of Sciences | |
local.contributor.affiliation | Ren, Weijun, Chinese Academy of Sciences | |
local.contributor.affiliation | Lu, Teng, College of Science, ANU | |
local.contributor.affiliation | Liu, Yun, College of Science, ANU | |
local.contributor.affiliation | Guo, Shaobo, Chinese Academy of Sciences | |
local.contributor.affiliation | Dong, Xianlin, Chinese Academy of Sciences | |
local.contributor.affiliation | Wang, Genshui, Chinese Academy of Sciences | |
local.bibliographicCitation.issue | 14 | |
local.bibliographicCitation.startpage | 1 | |
local.bibliographicCitation.lastpage | 5 | |
local.identifier.doi | 10.1063/1.5020424 | |
local.identifier.absseo | 970102 - Expanding Knowledge in the Physical Sciences | |
dc.date.updated | 2019-03-31T07:18:53Z | |
local.identifier.scopusID | 2-s2.0-85045017380 | |
dcterms.accessRights | Open Access | |
dc.provenance | http://sherpa.ac.uk/romeo/issn/0003-6951/..."Publishers version/PDF may be used on author's personal website, arXiv, institutional website, institutional repository, funders designated repository or private forums on social academic network after 12 months embargo" from SHERPA/RoMEO site (as at 11/07/19). | |
Collections | ANU Research Publications |
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