Energy dependence of p+232 Th fission mass distributions: Mass-asymmetric standard I and standard II modes, and multichance fission

Abstract

Background: The predominant mass-asymmetric fission of actinide nuclides occurs mainly through the so- called standard I and standard II modes. Though understood to be caused by shape-dependent shell structures encountered between the fission barrier deformation and scission, the most relevant shell gaps are still not firmly established. The standard I mode had been associated with the spherical doubly magic 132 Sn, and thus the Z = 50 proton shell, but recently it has been proposed that standard I and standard II are associated with quadrupole and octupole deformed gaps at Z = 52 and 56, respectively.

Purpose: We investigate how the relative probabilities of the standard I and standard II modes vary with excitation energy near threshold, probing where the two modes bifurcate.

Methods: The Australian National University Heavy Ion Accelerator Facility and CUBE fission spectrometer have been used to measure fission mass distributions for the p +232 Th reaction (forming 233 Pa) at closely spaced bombarding energy intervals from 6.5 to 28 MeV.

Results: A model-independent analysis of the energy dependence of the shape of the mass-asymmetric peak shows a strong dependence of the standard I and standard II relative probability on excitation energy near threshold.

Conclusions: The results are consistent with the standard II mode having a lower fission barrier than standard I in 233 Pa, with the latter increasing continually in relative probability above its barrier energy. It is concluded that multichance fission, in particular last chance fission, plays a strong role in determining the observed energy dependence of all fission modes.