Koch, WernerFrankcombe, Terry2015-12-130031-9007http://hdl.handle.net/1885/73148A wide variety of molecular systems that have recently come into the reach of experimental and theoretical investigation is dominated by quantum phenomena. However, even state of the art quantum propagation techniques are either unsuitable for general appAuthor/s retain copyrightKeywords: 3 degrees of freedom; Computational resources; General applications; Quantum phenomena; Quantum propagation; Strong interference; Theoretical investigations; Tunneling characteristics; Mechanics; Quantum theoryBasis expansion leaping: A new method to solve the time-dependent Schrödinger equation for molecular quantum dynamics201310.1103/PhysRevLett.110.2632022016-02-24