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Revealing the two-electron cusp in the ground states of He and H2 via quasifree double photoionization

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Authors

Grundmann, S
Serov, V V
Trinter, Florian
Fehre, Kilian
Strenger, Nico
Pier, Andreas
Kircher, Max
Trabert, Daniel
Weller, Miriam
Rist, Jonas

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American Physical Society

Abstract

We report on kinematically complete measurements and ab initio nonperturbative calculations of double ionization of He and H 2 by a single 800 eV circularly polarized photon. We confirm the quasifree mechanism of photoionization for H 2 and show how it originates from the two-electron cusp in the ground state of a two-electron target. Our approach establishes a method for mapping electrons relative to each other and provides valuable insight into photoionization beyond the electric-dipole approximation.

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Physical Review Research

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Open Access

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Creative Commons Attribution 4.0 International license

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