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A Chemoenzymatic Total Synthesis of the Phytotoxic Undecenolide (-)-Cladospolide A

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Banwell, Martin; Loong, David

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An eleven-step synthesis of the title compound (1) from biocatalytically-derived and enantiomerically pure 'building blocks' alcohol (R)-(-)-9 and ester 13 is described. Attempts to construct the twelve-membered lactone ring of cladospolide A in a direct

dc.contributor.authorBanwell, Martin
dc.contributor.authorLoong, David
dc.date.accessioned2015-12-13T22:41:19Z
dc.date.available2015-12-13T22:41:19Z
dc.identifier.issn1477-0520
dc.identifier.urihttp://hdl.handle.net/1885/78452
dc.description.abstractAn eleven-step synthesis of the title compound (1) from biocatalytically-derived and enantiomerically pure 'building blocks' alcohol (R)-(-)-9 and ester 13 is described. Attempts to construct the twelve-membered lactone ring of cladospolide A in a direct
dc.publisherRoyal Society of Chemistry
dc.sourceOrganic and Biomolecular Chemistry
dc.subjectKeywords: Biocatalysts; Chromatography; Enzymes; Filtration; Hydrogenation; Stereochemistry; Synthesis (chemical); X ray analysis; Allylic alcohols; Necrosis; Retrosynthetic analysis; Ring-closing metathesis (RCM); Amino acids; Alia; cladospolide a; cladospolide B;
dc.titleA Chemoenzymatic Total Synthesis of the Phytotoxic Undecenolide (-)-Cladospolide A
dc.typeJournal article
local.description.notesImported from ARIES
local.description.refereedYes
local.identifier.citationvolume2
dc.date.issued2004
local.identifier.absfor030503 - Organic Chemical Synthesis
local.identifier.ariespublicationMigratedxPub7093
local.type.statusPublished Version
local.contributor.affiliationBanwell, Martin, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationLoong, David, College of Physical and Mathematical Sciences, ANU
local.bibliographicCitation.issue14
local.bibliographicCitation.startpage2050
local.bibliographicCitation.lastpage2060
local.identifier.doi10.1039/b401829j
dc.date.updated2015-12-11T10:00:45Z
local.identifier.scopusID2-s2.0-3843132928
CollectionsANU Research Publications

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