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Exploiting multiple nucleophilic sites on pyrrole for the assembly of polyheterocyclic frameworks: application to a formal total synthesis of (±)-aspidospermidine

Banwell, Martin; Smith, Jason A

Description

The tricyclic ketone 19, an advanced intermediate in Aubé's recently reported synthesis of aspidospermidine (4), is prepared in twelve steps from pyrrole (3). The key transformations involve a previously described intramolecular Michael addition reaction

CollectionsANU Research Publications
Date published: 2002
Type: Journal article
URI: http://hdl.handle.net/1885/72397
Source: Journal of the Chemical Society, Perkin Transactions 1

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