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Total syntheses of the furanosesquiterpenes crassifolone and dihydrocrassifolone via an Au(I)-catalysed intramolecular Michael addition reaction

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Menon, Rajeev; Banwell, Martin

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The racemic modifications of title natural products 1 and 2 have been synthesised for the first time. The key step was the Au(i)-catalysed conversion of the furanyl-substituted ynone 13 into the annulated furan 14.

dc.contributor.authorMenon, Rajeev
dc.contributor.authorBanwell, Martin
dc.date.accessioned2015-12-10T22:41:18Z
dc.identifier.issn1477-0520
dc.identifier.urihttp://hdl.handle.net/1885/57835
dc.description.abstractThe racemic modifications of title natural products 1 and 2 have been synthesised for the first time. The key step was the Au(i)-catalysed conversion of the furanyl-substituted ynone 13 into the annulated furan 14.
dc.publisherRoyal Society of Chemistry
dc.sourceOrganic and Biomolecular Chemistry
dc.subjectKeywords: Dihydrocrassifolone; Furanosesquiterpenes; Intramolecular Michael addition; Natural products; Total synthesis; Addition reactions; Essential oils; Catalysis; benzofuran derivative; gold; sesquiterpene; article; catalysis; chemical structure; chemistry; sy
dc.titleTotal syntheses of the furanosesquiterpenes crassifolone and dihydrocrassifolone via an Au(I)-catalysed intramolecular Michael addition reaction
dc.typeJournal article
local.description.notesImported from ARIES
local.identifier.citationvolume8
dc.date.issued2010
local.identifier.absfor030503 - Organic Chemical Synthesis
local.identifier.ariespublicationu4005981xPUB417
local.type.statusPublished Version
local.contributor.affiliationMenon, Rajeev, College of Physical and Mathematical Sciences, ANU
local.contributor.affiliationBanwell, Martin, College of Physical and Mathematical Sciences, ANU
local.description.embargo2037-12-31
local.bibliographicCitation.issue24
local.bibliographicCitation.startpage5483
local.bibliographicCitation.lastpage5485
local.identifier.doi10.1039/C0OB00487A
local.identifier.absseo970103 - Expanding Knowledge in the Chemical Sciences
dc.date.updated2016-02-24T10:23:42Z
local.identifier.scopusID2-s2.0-78649496730
local.identifier.thomsonID000284610600002
CollectionsANU Research Publications

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