Modulation of Third-Order Nonlinear Optical Properties by Backbone Modification of Polymeric Pillared-Layer Heterometallic Clusters
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Zhang, Chi; Cao, Yuan; Zhang, Jinfang; Meng, Suci; Matsumoto, Tsuyosh; Song, Yinglin; Ma, Jing; Chen, Zhaoxu; Tatsumi, Kazuyuki; Humphrey, Mark
Description
A study was conducted to demonstrate the synthesis of three structurally interesting polymeric heterothiometallic clusters with 3D pillar-layer- alternating honeycomb structure. The study observed that the connecting pillar ligands can modulate the NLO behavior of cluster polymers by π-electron delocalization. The study also used a density functional theory (DFT) calculations to determine the influence of bridging ligands on the electronic structure. It was observed during the study that the...[Show more]
Collections | ANU Research Publications |
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Date published: | 2008 |
Type: | Journal article |
URI: | http://hdl.handle.net/1885/38409 |
Source: | Advanced Materials |
DOI: | 10.1002/adma.200702645 |
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