Cross-Coupling for Cross-Conjugation: Practical Synthesis and Diels-Alder Reactions of Dendralenes
(Chemical Equation Presented) The parent dendralene and 2-substituted dendralenes are made easily through cross-coupling reactions. Contrary to some earlier reports, dendralene is sufficiently stable to be handled using standard synthetic methods. These compounds allow the one-step stereoselective construction of polycyclic frameworks through reactions with dienophiles. Site selectivity and stereoselectivity in Diels-Alder reactions with dienophiles are generally not influenced by the...[Show more]
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