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Facile syntheses of silver thioantimonates exhibiting second-harmonic generation responses and large birefringence

Yang, Gang; Jiang, Xingxing; Wu, Chao; Lin, Zheshuai; Huang, Zhipeng; Humphrey, Mark; Zhang, Chi


Two chalcogenide crystalline compounds, [enH ][Ag Sb S ] (en = ethylenediamine) and [enH][Ag SbS ], have been successfully synthesized by mild ionothermal and solvothermal means. [enH][Ag SbS ] crystallizes in the noncentrosymmetric (NCS) and polar space groupPc, and its linear and nonlinear optical (NLO) properties have been investigated for the first time. Second harmonic generation (SHG) measurements revealed that [enH][Ag SbS ] affords powder SHG performance values of 2.5 × KDP @1064 nm and...[Show more]

CollectionsANU Research Publications
Date published: 2021
Type: Journal article
Source: Dalton Transactions
DOI: 10.1039/d0dt04043f


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