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Efficient and Layer-Dependent Exciton Pumping across Atomically Thin Organic–Inorganic Type-I Heterostructures

Zhang, Linglong; Sharma, Ankur; Zhu, Yi; Zhang, Yuhan; Wang, Bowen; Dong, Miheng; Nguyen, Hieu; Wang, Zhu; Wen, Bo; Cao, Yujie; Liu, Boqing; Sun, Xueqian; Yang, Jiong; Li, Ziyuan; Kar, Arara; Shi, Yi; Macdonald, Daniel; Yu, Zongfu; Wang, Xinran; Lu, Yuerui


The fundamental light–matter interactions in monolayer transition metal dichalcogenides might be significantly engineered by hybridization with their organic counterparts, enabling intriguing optoelectronic applications. Here, atomically thin organic–inorganic (O–I) heterostructures, comprising monolayer MoSe2 and mono‐/few‐layer single‐crystal pentacene samples, are fabricated. These heterostructures show type‐I band alignments, allowing efficient and layer‐dependent exciton pumping across the...[Show more]

CollectionsANU Research Publications
Date published: 2018-08-30
Type: Journal article
Source: Advanced Materials
DOI: 10.1002/adma.201803986
Access Rights: Open Access


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