Toward a Quantitative Description of Radical Photoinitiator Structure–Reactivity Correlations
The fundamental influence of the structure and substitution of radical photoinitiators was investigated via a trifold combination of pulsedlaser polymerization with subsequent electrospray-ionization mass spectrometry (PLP-ESI-MS), femtosecond transient absorption (fs-TA) spectroscopy, and quantum chemistry. For the first time, a library of benzoin-derived photoinitiators with varied substitution patterns was synthesized. In the PLPESI-MS study, different photoinitiators were compared...[Show more]
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