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Isolated Diatomic Ni-Fe Metal-Nitrogen Sites for Synergistic Electroreduction of CO2

Ren, Wenhao; Tan, Xin; Yang, Wanfeng; Jia, Chen; Xu, Shumao; Wang, Kaixue; Smith, Sean; Zhao, Chuan


Polynary single‐atom structures can combine the advantages of homogeneous and heterogeneous catalysts while providing synergistic functions based on different molecules and their interfaces. However, the fabrication and identification of such an active‐site prototype remain elusive. Here we report isolated diatomic Ni‐Fe sites anchored on nitrogenated carbon as an efficient electrocatalyst for CO2 reduction. The catalyst exhibits high selectivity with CO Faradaic efficiency above 90 % over a...[Show more]

CollectionsANU Research Publications
Date published: 2019-04-17
Type: Journal article
Source: Angewandte Chemie International Edition
DOI: 10.1002/anie.201901575
Access Rights: Open Access


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