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Predissociation mechanism for the lowest ¹Πu states of N₂

Lewis, B. R.; Gibson, S. T.; Zhang, W.; Lefebvre-Brion, H.; Robbe, J.-M.


Separate coupled-channel Schrödinger-equation (CSE) models of the interacting ¹Πu (b,c,o) and ³Πu (C,C′) states of N₂ are combined, through the inclusion of spin-orbit interactions, to produce a five-channel CSE model of the N₂predissociation. Comparison of the model calculations with an experimental database, consisting principally of detailed new measurements of the vibrational and isotopic dependence of the Πu1linewidths and lifetimes, provides convincing evidence that the predissociation of...[Show more]

CollectionsANU Research Publications
Date published: 2005
Type: Journal article
Source: The Journal of Chemical Physics
DOI: 10.1063/1.1869986


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