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Linear Optical and Third-Order Nonlinear Optical Properties of Some Fluorenyl- and Triarylamine-Containing Tetracyanobutadiene Derivatives

Pokladek, Ziemowit; Ripoche, Nicolas; Betou, Marie; Trolez, Yann; Mongin, Olivier; Olesiak-Banska, Joanna; Matczyszyn, Katarzyna; Samoc, Marek; Humphrey, Mark; Blanchard-Desce, Mireille; Paul, Frédéric


The synthesis and characterization of four new tetracyanobutadiene (TCBD) derivatives (1-3 and 2') incorporating 2- or 2,7-fluorenyl and diphenylamino moieties are reported. The electroactivity of 1-3 and 2' was studied by cyclic voltammetry (CV), while the linear optical and (third-order) nonlinear optical (NLO) properties were investigated by electronic spectroscopy and Z-scan studies, respectively. All experimental investigations were rationalized by DFT computations, providing an insight...[Show more]

CollectionsANU Research Publications
Date published: 2016-07-11
Type: Journal article
Source: Chemistry - A European Journal
DOI: 10.1002/chem.201600897
Access Rights: Open Access


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