The Application of Pericyclic, Photolytic, Chemoenzymatic and Cross-coupling Techniques to the Synthesis of Biologically Active Natural Products and Related Structures
The body of this thesis is comprised of four scientific articles and is preceded by an overview that contextualises all of this submitted/published work. The first major part of this thesis is comprised of Publication 1. This details work concerned with establishing the true structure of the sorbicillinoid-derived isolate rezishanone C by total synthesis. Specifically, the enantiomer of what proved to be the true structure of the sorbicillinoid rezishanone C (sorbivinetone) was synthesized...[Show more]
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