A one-pot route to thioamides discovered by gas-phase studies

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Noor, Asif
Li, Jiawei
Khairallah, George N.
Li, Zhen
Ghari, Hossein
Canty, Allan J.
Ariafard, Alireza
Donnelly, Paul S.
O'Hair, Richard A.J.

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A new palladium mediated “one pot” synthesis of thioamides from aromatic carboxylic acids (ArCO2H + RNCS → ArC(S)NHR + CO2) was discovered by gas-phase experiments and theoretical studies. Palladium-mediated decarboxylation of aromatic carboxylic acids followed by addition of substituted isothiocyanates leads to the corresponding thioamide derivatives.

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Chemical Communications

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