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Ruthenium clusters with nitrogen ligands IV. Double CH activation of ketimine methyl groups on triruthenium carbonyl clusters. Crystal structure of Ru<sub>3</sub>(μ-H)<sub>2</sub>[μ<sub>3</sub>-ν<sup>2</sup>-(N,C)-4-HOC<sub>6</sub>H<sub>4</sub>NCMeCH](CO)<sub>9</sub>. Et<sub>2</sub>0

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Cifuentes, Marie P.
Jeynes, Tyrone P.
Gray, Matthew
Humphrey, Mark G.
Skelton, Brian W.
White, Allan H.

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The reaction of Ru3(CO)12 with the Schiff base 4-hydroxyphenyl-N,N-dimethylimide in refluxing cyclohexane gave the title complex in excellent yield. An X-ray crystallographic study showed that the product is derived from an unusual double CH activation of the methyl group. An analogous reaction with the asymmetric Schiff base p-hydroxyphenyl-N,N-isobutylmethylimide showed that this reaction is specific for the imine-bound methyl group.

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Journal of Organometallic Chemistry

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