Synthesis and Exfoliation of a New Layered Mesoporous Zr-MOF Comprising Hexa- A nd Dodecanuclear Clusters as Well as a Small Organic Linker Molecule

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Leubner, Sebastian
Bengtsson, Viktor E.G.
Synnatschke, Kevin
Gosch, Jonas
Koch, Alexander
Reinsch, Helge
Xu, Hongyi
Backes, Claudia
Zou, Xiaodong
Stock, Norbert

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A new layered mesoporous Zr-MOF of composition [Zr30O20(OH)26(OAc)18L18] was synthesized by employing 5-acetamidoisophthalic acid (H2L) using acetic acid as the solvent. The new MOF, denoted as CAU-45, exhibits a honeycomb structure of stacked layers which comprise both hexa- A nd dodecanucelar zirconium clusters. Its structure was solved from submicrometer-sized crystals by continuous rotation electron diffraction (cRED). Liquid phase exfoliation and size selection were successfully performed on the material.

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Journal of the American Chemical Society

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